Changes on the nanostructure of cementitius calcium silicate hydrates (C–S–H) induced by aqueous carbonation
نویسندگان
چکیده
منابع مشابه
Nanostructure of calcium silicate hydrates in cements.
Calcium silicate hydrate (CSH) is the major volume phase in the matrix of Portland cement concrete. Total x-ray scattering measurements with synchrotron x rays on synthetic CSH(I) shows nanocrystalline ordering with a particle diameter of 3.5(5) nm, similar to a size-broadened 1.1 nm tobermorite crystal structure. The CSH component in hydrated tricalcium silicate is found to be similar to CSH(I...
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15 صفحه اولFactors Affecting Ex-Situ Aqueous Mineral Carbonation Using Calcium and Magnesium Silicate Minerals
Carbonation of magnesiumand calcium-silicate minerals to form their respective carbonates is one method to sequester carbon dioxide. Process development studies have identified reactor design as a key component affecting both the capital and operating costs of ex-situ mineral sequestration. Results from mineral carbonation studies conducted in a batch autoclave were utilized to design and const...
متن کاملIntermolecular Forces Between Nanolayers of Crystalline Calcium-Silicate-Hydrates in Aqueous Medium
Calcium-silicate-hydrate (C-S-H) is the major binding phase responsible for strength and durability of cementitious materials. The cohesive properties of C-S-H are directly related to the intermolecular forces between its layers at the nanoscale. Here, we employ free energy perturbation theory (FEP) to calculate intermolecular forces between crystalline C-S-H layers solvated in aqueous medium a...
متن کاملThermodynamics of water confined in porous calcium-silicate-hydrates.
Water within pores of cementitious materials plays a crucial role in the damage processes of cement pastes, particularly in the binding material comprising calcium-silicate-hydrates (C-S-H). Here, we employed Grand Canonical Monte Carlo simulations to investigate the properties of water confined at ambient temperature within and between C-S-H nanoparticles or "grains" as a function of the relat...
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ژورنال
عنوان ژورنال: Journal of Materials Science
سال: 2011
ISSN: 0022-2461,1573-4803
DOI: 10.1007/s10853-011-5852-6